Atmospheric dispersion modeling
Atmospheric dispersion modeling is the mathematical simulation of how air pollutants disperse in the ambient atmosphere. It is performed with computer programs that include algorithms to solve the mathematical equations that govern the pollutant dispersion. The dispersion models are used to estimate the downwind ambient concentration of air pollutants or toxins emitted from sources such as industrial plants, vehicular traffic or accidental chemical releases. They can also be used to predict future concentrations under specific scenarios (i.e. changes in emission sources). Therefore, they are the dominant type of model used in air quality policy making. They are most useful for pollutants that are dispersed over large distances and that may react in the atmosphere. For pollutants that have a very high spatio-temporal variability (i.e. have very steep distance to source decay such as black carbon) and for epidemiological studies statistical land-use regression models are also used.
Dispersion models are important to governmental agencies tasked with protecting and managing the ambient air quality. The models are typically employed to determine whether existing or proposed new industrial facilities are or will be in compliance with the National Ambient Air Quality Standards (NAAQS) in the United States and other nations. The models also serve to assist in the design of effective control strategies to reduce emissions of harmful air pollutants. During the late 1960s, the Air Pollution Control Office of the U.S. EPA initiated research projects that would lead to the development of models for the use by urban and transportation planners.[1] A major and significant application of a roadway dispersion model that resulted from such research was applied to the Spadina Expressway of Canada in 1971.
Air dispersion models are also used by public safety responders and emergency management personnel for emergency planning of accidental chemical releases. Models are used to determine the consequences of accidental releases of hazardous or toxic materials, Accidental releases may result in fires, spills or explosions that involve hazardous materials, such as chemicals or radionuclides. The results of dispersion modeling, using worst case accidental release source terms and meteorological conditions, can provide an estimate of location impacted areas, ambient concentrations, and be used to determine protective actions appropriate in the event a release occurs. Appropriate protective actions may include evacuation or shelter in place for persons in the downwind direction. At industrial facilities, this type of consequence assessment or emergency planning is required under the U.S. Clean Air Act (CAA) codified in Part 68 of Title 40 of the Code of Federal Regulations.
The dispersion models vary depending on the mathematics used to develop the model, but all require the input of data that may include:
Many of the modern, advanced dispersion modeling programs include a pre-processor module for the input of meteorological and other data, and many also include a post-processor module for graphing the output data and/or plotting the area impacted by the air pollutants on maps. The plots of areas impacted may also include isopleths showing areas of minimal to high concentrations that define areas of the highest health risk. The isopleths plots are useful in determining protective actions for the public and responders.
The atmospheric dispersion models are also known as atmospheric diffusion models, air dispersion models, air quality models, and air pollution dispersion models.
Atmospheric layers[edit]
Discussion of the layers in the Earth's atmosphere is needed to understand where airborne pollutants disperse in the atmosphere. The layer closest to the Earth's surface is known as the troposphere. It extends from sea-level to a height of about 18 km (11 mi) and contains about 80 percent of the mass of the overall atmosphere. The stratosphere is the next layer and extends from 18 km (11 mi) to about 50 km (31 mi). The third layer is the mesosphere which extends from 50 km (31 mi) to about 80 km (50 mi). There are other layers above 80 km, but they are insignificant with respect to atmospheric dispersion modeling.
The lowest part of the troposphere is called the planetary boundary layer (PBL), or sometimes the atmospheric boundary layer. The air temperature of the PBL decreases with increasing altitude until it reaches a capping inversion, which is a type of inversion layer where warmer air sits higher in the atmosphere than cooler air. We call the region of the PBL below its capping inversion the convective planetary boundary layer; it is typically 1.5 to 2 km (0.93 to 1.24 mi) in height. The upper part of the troposphere (i.e., above the inversion layer) is called the free troposphere and it extends up to the tropopause (the boundary in the Earth's atmosphere between the troposphere and the stratosphere). In tropical and mid-latitudes during daytime, the free convective layer can comprise the entire troposphere, which is up to 10 to 18 km (6.2 to 11.2 mi) in the intertropical convergence zone.
The PBL is important with respect to the transport and dispersion of airborne pollutants because the turbulent dynamics of wind are strongest at Earth's surface. The part of the PBL between the Earth's surface and the bottom of the inversion layer is known as the mixing layer. Almost all of the airborne pollutants emitted into the ambient atmosphere are transported and dispersed within the mixing layer. Some of the emissions penetrate the inversion layer and enter the free troposphere above the PBL.
In summary, the layers of the Earth's atmosphere from the surface of the ground upwards are: the PBL made up of the mixing layer capped by the inversion layer; the free troposphere; the stratosphere; the mesosphere and others. Many atmospheric dispersion models are referred to as boundary layer models because they mainly model air pollutant dispersion within the ABL. To avoid confusion, models referred to as mesoscale models have dispersion modeling capabilities that extend horizontally up to a few hundred kilometres. It does not mean that they model dispersion in the mesosphere.
The Gaussian air pollutant dispersion equation (discussed above) requires the input of H which is the pollutant plume's centerline height above ground level—and H is the sum of Hs (the actual physical height of the pollutant plume's emission source point) plus ΔH (the plume rise due to the plume's buoyancy).
To determine ΔH, many if not most of the air dispersion models developed between the late 1960s and the early 2000s used what are known as the Briggs equations. G.A. Briggs first published his plume rise observations and comparisons in 1965.[9] In 1968, at a symposium sponsored by CONCAWE (a Dutch organization), he compared many of the plume rise models then available in the literature.[10] In that same year, Briggs also wrote the section of the publication edited by Slade[11] dealing with the comparative analyses of plume rise models. That was followed in 1969 by his classical critical review of the entire plume rise literature,[12] in which he proposed a set of plume rise equations which have become widely known as "the Briggs equations". Subsequently, Briggs modified his 1969 plume rise equations in 1971 and in 1972.[13][14]
Briggs divided air pollution plumes into these four general categories:
Briggs considered the trajectory of cold jet plumes to be dominated by their initial velocity momentum, and the trajectory of hot, buoyant plumes to be dominated by their buoyant momentum to the extent that their initial velocity momentum was relatively unimportant. Although Briggs proposed plume rise equations for each of the above plume categories, it is important to emphasize that "the Briggs equations" which become widely used are those that he proposed for bent-over, hot buoyant plumes.
In general, Briggs's equations for bent-over, hot buoyant plumes are based on observations and data involving plumes from typical combustion sources such as the flue gas stacks from steam-generating boilers burning fossil fuels in large power plants. Therefore, the stack exit velocities were probably in the range of 20 to 100 ft/s (6 to 30 m/s) with exit temperatures ranging from 250 to 500 °F (120 to 260 °C).
A logic diagram for using the Briggs equations[4] to obtain the plume rise trajectory of bent-over buoyant plumes is presented below:
The above parameters used in the Briggs' equations are discussed in Beychok's book.[4]
See also[edit]
Atmospheric dispersion models[edit]
List of atmospheric dispersion models provides a more comprehensive list of models than listed below. It includes a very brief description of each model.